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Resonant photocurrent from a single quantum emitter in tungsten diselenide

Authors :
Matthias Paur
Aday J. Molina-Mendoza
Dmitry K. Polyushkin
Thomas Mueller
Rudolf Bratschitsch
Steffen Michaelis de Vasconcellos
Source :
2D Materials. 7:045021
Publication Year :
2020
Publisher :
IOP Publishing, 2020.

Abstract

Single quantum emitters (SQEs) are the basic building blocks for quantum optics and quantum information technology. Strain-induced defects in monolayer transition metal dichalcogenides (TMDs) have been shown to be a promising platform for the generation of SQEs. In particular, achieving optically active and electrically controlled quantum emitters make these materials attractive for applications ranging from quantum communication and optoelectronics to high resolution metrology. Here, we report the spectral photoresponse of monolayer WSe2 upon strain, where we observe a connection between single-photon emission and photocurrent (PC) generation in a p-n device. A strong antibunching in second-order correlation from this localized emitter unambiguously demonstrates the single-photon nature of the emission, whereas the PC is highly dominated by the absorption at such a localized state, showing an exponential dependence with the applied electric field. Furthermore, we can resolve narrow PC peaks with 1.0 meV spectral width.

Details

ISSN :
20531583
Volume :
7
Database :
OpenAIRE
Journal :
2D Materials
Accession number :
edsair.doi...........35294ce3b7a2e5a18bcf835beabb6650
Full Text :
https://doi.org/10.1088/2053-1583/aba4ec