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Evolution of the metallic state in LaNiO3/LaAlO3 superlattices measured by Li8β -detected NMR

Authors :
Bernhard Keimer
Georg Cristiani
Gennady Logvenov
W. Andrew MacFarlane
Gerald D. Morris
Victoria L. Karner
Aris Chatzichristos
Ryan M. L. McFadden
Derek Fujimoto
Ruohong Li
C. D. Philip Levy
Eva Benckiser
Robert F. Kiefl
Matthew Pearson
David L Cortie
Alexander Boris
Source :
Physical Review B. 104
Publication Year :
2021
Publisher :
American Physical Society (APS), 2021.

Abstract

Using ion-implanted $^{8}\mathrm{Li} \ensuremath{\beta}$-detected NMR, we study the evolution of the correlated metallic state of ${\mathrm{LaNiO}}_{3}$ in a series of ${\mathrm{LaNiO}}_{3}/{\mathrm{LaAlO}}_{3}$ superlattices as a function of bilayer thickness. Spin-lattice relaxation measurements in an applied field of $6.55\phantom{\rule{0.16em}{0ex}}\mathrm{T}$ reveal two equal amplitude components: one with metallic ($T$ linear) $1/{T}_{1}$ and a second with a more complex $T$ dependence. The metallic character of the slow relaxing component is only weakly affected by the ${\mathrm{LaNiO}}_{3}$ thickness, while the fast component is much more sensitive, exhibiting the opposite temperature dependence (increasing toward low $T$) in the thinnest, most magnetic samples. The origin of this bipartite relaxation is discussed in terms of electronic phase separation.

Details

ISSN :
24699969 and 24699950
Volume :
104
Database :
OpenAIRE
Journal :
Physical Review B
Accession number :
edsair.doi...........2762b6aa4c7fe9e27e2290ea0c58a9cf
Full Text :
https://doi.org/10.1103/physrevb.104.205114