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The First Total Synthesis of Pectinolide F

Authors :
Gowravaram Sabitha
Jhillu S. Yadav
Chevula Gurumurthy
Source :
Synthesis. 46:1757-1764
Publication Year :
2014
Publisher :
Georg Thieme Verlag KG, 2014.

Abstract

The first total synthesis of the natural saturated α-pyrone pectinolide F has been accomplished from inexpensive, commercially available ( S )-ethyl lactate and but-3-yn-1-ol. The salient features of the synthesis are 2,2,6,6-tetramethylpiperidin-1-oxyl (TEMPO)–[bis(acetoxy)iodo]benzene oxidation, Sharpless asymmetric dihydroxylation, Grignard reaction, and partial hydrogenation of the triple bond.

Details

ISSN :
1437210X and 00397881
Volume :
46
Database :
OpenAIRE
Journal :
Synthesis
Accession number :
edsair.doi...........151a6e23cac3669feff56ba720a9bc45