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Infrared Interlayer Exciton Emission in MoS2/WSe2 Heterostructures

Authors :
Eric Yue Ma
Janina Maultzsch
Elyse Barré
Ralph H. Page
Kenji Watanabe
Bumho Kim
Tony F. Heinz
Ouri Karni
Sze Cheung Lau
Takashi Taniguchi
Katayun Barmak
Roland Gillen
Source :
Physical Review Letters. 123
Publication Year :
2019
Publisher :
American Physical Society (APS), 2019.

Abstract

We report light emission around 1 eV (1240 nm) from heterostructures of MoS_{2} and WSe_{2} transition metal dichalcogenide monolayers. We identify its origin in an interlayer exciton (ILX) by its wide spectral tunability under an out-of-plane electric field. From the static dipole moment of the state, its temperature and twist-angle dependence, and comparison with electronic structure calculations, we assign this ILX to the fundamental interlayer transition between the K valleys in this system. Our findings gain access to the interlayer physics of the intrinsically incommensurate MoS_{2}/WSe_{2} heterostructure, including moire and valley pseudospin effects, and its integration with silicon photonics and optical fiber communication systems operating at wavelengths longer than 1150 nm.

Details

ISSN :
10797114 and 00319007
Volume :
123
Database :
OpenAIRE
Journal :
Physical Review Letters
Accession number :
edsair.doi...........072caf700b69164e6423e150a44f314c