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Correlated surface bands of the prototypical interface Sn/Si-alphaR3

Authors :
Charrier, Anne
Pérez, R
Thibaudau, F.
Debever, J.-M
Ortega, J
Flores, F
Themlin, J.-M
Centre Interdisciplinaire de Nanoscience de Marseille (CINaM)
Aix Marseille Université (AMU)-Centre National de la Recherche Scientifique (CNRS)
Centre de recherche de la matière condensée et des nanosciences (CRMCN)
Université de la Méditerranée - Aix-Marseille 2-Université Paul Cézanne - Aix-Marseille 3-Centre National de la Recherche Scientifique (CNRS)
Centre National de la Recherche Scientifique (CNRS)-Aix Marseille Université (AMU)
CHARRIER, Anne
Source :
Applied Surface Science, Applied Surface Science, 2001, Applied Surface Science, Elsevier, 2001
Publication Year :
2001
Publisher :
HAL CCSD, 2001.

Abstract

International audience; Using angle-resolved inverse photoemission spectroscopy (KRIPES), we have investigated the unoccupied electronic structure of the model interface Sn/Si(1 1 1)-a-  3 p at room temperature. In addition to a ``metallic'' surface state crossing the Fermi level (E F) near the K H point, we unambiguously assign a second feature of our KRIPES spectra, located around 1.5 eV above E F , to a second surface state U H 2. We will experimentally show that U H 2 is an intrinsic feature of the a-  3 p reconstruction which cannot be associated with defects. The existence of these two surface states is not compatible with the ideal T 4 model which would show either a single, half-occupied metallic band crossing E F , or an insulating phase if strong correlation effects, important for these narrow surface bands, are considered. Rather, both U H 1 and U H 2 receive a natural explanation, once many-body effects are introduced, in the framework of a dynamical ¯uctuations model, where two kinds of Sn adatoms sites reminiscent of a low-temperature 3  3 phase do persist at room temperature. Correlated surface bands incorporating many-body effects in a non restricted way provide a complete description of the experimental surface bands and their dispersions. #

Details

Language :
English
ISSN :
01694332
Database :
OpenAIRE
Journal :
Applied Surface Science, Applied Surface Science, 2001, Applied Surface Science, Elsevier, 2001
Accession number :
edsair.dedup.wf.001..90de4b247aa4665e6fc80084f404eb9d