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Stable continuous-wave lasing from discrete cesium lead bromide quantum dots embedded in a microcavityElectronic supplementary information (ESI) available. See DOI: https://doi.org/10.1039/d3nh00139c
- Source :
- Nanoscale Horizons; 2023, Vol. 8 Issue: 10 p1403-1410, 8p
- Publication Year :
- 2023
-
Abstract
- All-inorganic cesium lead bromide (CsPbBr3) quantum dots (QDs) with high photoluminescence (PL) quantum efficiency have been reported as ideal gain materials for high-performance lasers. Nevertheless, isolated CsPbBr3QDs have not achieved lasing emission (LE) due to finite absorption cross-section. Here, we demonstrate continuous-wave lasing of isolated CsPbBr3QDs embedded in a microcavity. Distributed Bragg reflectors (DBRs), together with isolated CsPbBr3QDs in a polymer matrix, are introduced to construct a vertical-cavity surface-emitting laser (VCSEL), which exhibits stable single-mode lasing emissions with an ultra-low threshold of 8.8 W cm−2and a high Qfactor of 1787. Such perovskite-based microcavity structures sustain highly stable excitons at room temperature and can provide an excellent experimental platform to further study the single-particle nano-lasers and quantum physics frontiers such as exciton–polariton condensation, single-photon emission, and optical quantum communication.
Details
- Language :
- English
- ISSN :
- 20556756 and 20556764
- Volume :
- 8
- Issue :
- 10
- Database :
- Supplemental Index
- Journal :
- Nanoscale Horizons
- Publication Type :
- Periodical
- Accession number :
- ejs64051750
- Full Text :
- https://doi.org/10.1039/d3nh00139c