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Stable continuous-wave lasing from discrete cesium lead bromide quantum dots embedded in a microcavityElectronic supplementary information (ESI) available. See DOI: https://doi.org/10.1039/d3nh00139c

Authors :
Zhang, Hongbo
Wen, Wen
Du, Bowen
Zhou, Lei
Chen, Yu
Feng, Shun
Zou, Chenji
Wu, Lishu
Fan, Hong Jin
Gao, Weibo
Sun, Handong
Shang, Jingzhi
Yu, Ting
Source :
Nanoscale Horizons; 2023, Vol. 8 Issue: 10 p1403-1410, 8p
Publication Year :
2023

Abstract

All-inorganic cesium lead bromide (CsPbBr3) quantum dots (QDs) with high photoluminescence (PL) quantum efficiency have been reported as ideal gain materials for high-performance lasers. Nevertheless, isolated CsPbBr3QDs have not achieved lasing emission (LE) due to finite absorption cross-section. Here, we demonstrate continuous-wave lasing of isolated CsPbBr3QDs embedded in a microcavity. Distributed Bragg reflectors (DBRs), together with isolated CsPbBr3QDs in a polymer matrix, are introduced to construct a vertical-cavity surface-emitting laser (VCSEL), which exhibits stable single-mode lasing emissions with an ultra-low threshold of 8.8 W cm−2and a high Qfactor of 1787. Such perovskite-based microcavity structures sustain highly stable excitons at room temperature and can provide an excellent experimental platform to further study the single-particle nano-lasers and quantum physics frontiers such as exciton–polariton condensation, single-photon emission, and optical quantum communication.

Details

Language :
English
ISSN :
20556756 and 20556764
Volume :
8
Issue :
10
Database :
Supplemental Index
Journal :
Nanoscale Horizons
Publication Type :
Periodical
Accession number :
ejs64051750
Full Text :
https://doi.org/10.1039/d3nh00139c