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Electroluminescence and Plasmon-Assisted Directional Photoluminescence from 2D HgTe Nanoplatelets

Authors :
Dabard, Corentin
Bossavit, Erwan
Dang, Tung Huu
Ledos, Nicolas
Cavallo, Mariarosa
Khalili, Adrien
Zhang, Huichen
Alchaar, Rodolphe
Patriarche, Gilles
Vasanelli, Angela
Diroll, Benjamin T.
Degiron, Aloyse
Lhuillier, Emmanuel
Ithurria, Sandrine
Source :
The Journal of Physical Chemistry - Part C; 20230101, Issue: Preprints
Publication Year :
2023

Abstract

In the visible range, 2D nanoplatelets (NPLs) have brought significant benefits compared to their 0D counterpart with an inherently anisotropic emission, a narrower photoluminescence (PL) signal, and new degrees of freedom to design heterostructures. Compared to the properties of cadmium chalcogenide NPLs in the visible, similar research is still mostly lacking in the infrared, in spite of existing synthetic paths to obtain narrow band gap semiconductors in 2D colloidal form. Here, we focus on 2D HgTe NPLs and show how their PL can be stabilized through the proper choice of surface chemistry. We then demonstrate two important steps toward bright infrared light emitting diodes (LEDs) which are (i) the coupling to a plasmonic grating to control the magnitude and spatial direction of the PL signal and (ii) the observation of electroluminescence at 1300 nm, which is near telecom wavelength.

Details

Language :
English
ISSN :
19327447 and 19327455
Issue :
Preprints
Database :
Supplemental Index
Journal :
The Journal of Physical Chemistry - Part C
Publication Type :
Periodical
Accession number :
ejs63614836
Full Text :
https://doi.org/10.1021/acs.jpcc.3c04126