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Optimizing the oxide support composition in Pr-doped CeO2towards highly active and selective Ni-based CO2methanation catalysts

Authors :
Tsiotsias, Anastasios I.
Charisiou, Nikolaos D.
AlKhoori, Ayesha
Gaber, Safa
Stolojan, Vlad
Sebastian, Victor
van der Linden, Bart
Bansode, Atul
Hinder, Steven J.
Baker, Mark A.
Polychronopoulou, Kyriaki
Goula, Maria A.
Source :
Journal of Energy Chemistry; August 2022, Vol. 71 Issue: 1 p547-561, 15p
Publication Year :
2022

Abstract

Pr doping of CeO2up to 10at% (Ce0.9Pr0.1O2-δ) in Ni/CeO2increases the oxygen vacancy population and reduces the Ni particle size, improving CO2methanation activity and lowering the activation energy.

Details

Language :
English
ISSN :
20954956
Volume :
71
Issue :
1
Database :
Supplemental Index
Journal :
Journal of Energy Chemistry
Publication Type :
Periodical
Accession number :
ejs59418567
Full Text :
https://doi.org/10.1016/j.jechem.2022.04.003