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Aerosol mass and black carbon concentrations, two year-round observations at NCO-P (5079 m, Southern Himalayas).

Authors :
Marinoni, A.
Cristofanelli, P.
Laj, P.
Duchi, R.
Calzolari, F.
Decesari, S.
Sellegri, K.
Vuillermoz, E.
Verza, G. P.
Villani, P.
Bonasoni, P.
Source :
Atmospheric Chemistry & Physics Discussions; 2010, Vol. 10 Issue 3, p8379-8413, 35p, 2 Charts, 6 Graphs
Publication Year :
2010

Abstract

Aerosol mass and the absorbing fraction are important variables, needed to constrain the role of atmospheric particles in the Earth radiation budget, both directly and indirectly through CCN activation. In particular, their monitoring in remote areas and mountain sites is essential for determining source regions, elucidating the mechanisms of long range transport of anthropogenic pollutants, and validating regional and global models. Since March 2006, aerosol mass and black carbon concentration have been monitored at the Nepal Climate Observatory-Pyramid, a permanent high-altitude research station located in the Khumbu valley at 5079ma.s.l. below Mt. Everest. The first 10 two-year averages of PM<subscript>1</subscript> and PM<subscript>1-10</subscript> mass were 1.94 μgm<superscript>-3</superscript> and 1.88 μgm<superscript>-3</superscript>, with standard deviations of 3.90 μgm<superscript>-3</superscript> and 4.45 μgm<superscript>-3</superscript>, respectively, while the black carbon concentration average is 160.5 ngm<superscript>-3</superscript>, with a standard deviation of 296.1 ngm<superscript>-3</superscript>. Both aerosol mass and black carbon show well defined annual cycles, with a maximum during the pre-monsoon season and a minimum during the monsoon. They also display a typical diurnal cycle during all the seasons, with the lowest particle concentration recorded during the night, and a considerable increase during the afternoon, revealing the major role played by thermal winds in influencing the behaviour of atmospheric compounds over the high Himalayas. The aerosol concentration is subject to high variability: in fact, as well as frequent "background conditions" (55% of the time) when BC concentrations are mainly below 100 ngm<superscript>-3</superscript>, concentrations up to 5 μgm<superscript>-3</superscript> are reached during some episodes (a few days every year) in the pre-monsoon seasons. The variability of PM and BC is the result of both short-term changes due to thermal wind development in the valley, and long-range transport/synoptic circulation. At NCO-P, higher concentrations of PM1 and BC are mostly associated with regional circulation and westerly air masses from the Middle East, while the strongest contributions of mineral dust arrive from the Middle East and regional circulation, with a special contribution from North Africa and South-West Arabian Peninsula in post-monsoon and winter season. [ABSTRACT FROM AUTHOR]

Details

Language :
English
ISSN :
16807367
Volume :
10
Issue :
3
Database :
Complementary Index
Journal :
Atmospheric Chemistry & Physics Discussions
Publication Type :
Academic Journal
Accession number :
49005935
Full Text :
https://doi.org/10.5194/acpd-10-8379-2010