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Dynamic correlations with time-dependent quantum Monte Carlo.

Authors :
Christov, Ivan P.
Source :
Journal of Chemical Physics; 6/28/2008, Vol. 128 Issue 24, p244106, 7p, 5 Graphs
Publication Year :
2008

Abstract

In this paper, we solve quantum many-body problem by propagating ensembles of trajectories and guiding waves in physical space. We introduce the “effective potential” correction within the recently proposed time-dependent quantum Monte Carlo methodology to incorporate the nonlocal quantum correlation effects between the electrons. The associated correlation length is calculated by adaptive kernel density estimation over the walker distribution. The general formalism is developed and tested on one-dimensional helium atom in laser field of different intensities and carrier frequencies. Good agreement with exact results for the atomic ionization is obtained. [ABSTRACT FROM AUTHOR]

Details

Language :
English
ISSN :
00219606
Volume :
128
Issue :
24
Database :
Complementary Index
Journal :
Journal of Chemical Physics
Publication Type :
Academic Journal
Accession number :
32990887
Full Text :
https://doi.org/10.1063/1.2943674