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High-performance Ag0.8Pb18+xSbTe20 thermoelectric bulk materials fabricated by mechanical alloying and spark plasma sintering.

High-performance Ag0.8Pb18+xSbTe20 thermoelectric bulk materials fabricated by mechanical alloying and spark plasma sintering.

Authors :
Heng Wang
Jing-Feng Li
Ce-Wen Nan
Min Zhou
Weishu Liu
Bo-Ping Zhang
Takuji Kita
Source :
Applied Physics Letters; 2/27/2006, Vol. 88 Issue 9, p092104, 3p, 1 Black and White Photograph, 1 Chart, 3 Graphs
Publication Year :
2006

Abstract

Polycrystalline Ag<subscript>n</subscript>Pb<subscript>m</subscript>SbTe<subscript>m+2n</subscript> thermoelectric materials, whose compositions can be described as Ag<subscript>0.8</subscript>Pb<subscript>18+x</subscript>SbTe<subscript>20</subscript> were prepared using a combined process of mechanical alloying and spark plasma sintering. Electric properties of the sintered samples with different Pb contents were measured from room temperature to 700 K. The maximum power factor of 1.766 mW/mK<superscript>2</superscript> was obtained at 673 K for the Ag<subscript>0.8</subscript>Pb<subscript>22</subscript>SbTe<subscript>20</subscript> sample, which corresponds to a high dimensionless figure of merit, ZT=1.37. This best composition is different from that reported before. [ABSTRACT FROM AUTHOR]

Details

Language :
English
ISSN :
00036951
Volume :
88
Issue :
9
Database :
Complementary Index
Journal :
Applied Physics Letters
Publication Type :
Academic Journal
Accession number :
20064703
Full Text :
https://doi.org/10.1063/1.2181197