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Modification of the Electrical Properties of a Bi0.8Ca0.2FeO3/LaNiO3/LaAlO3 Heterostructure: Effect of 80 MeV O+7 Ion Irradiation.

Authors :
Hajra, Sumana
Josely Jose, P.
Rathod, Urjitsinh I.
Keshvani, Mukesh
Sahoo, Jayaprakash
Vagadia, Megha
Meena, R.
Ojha, S.
Ravalia, Ashish
Source :
Journal of Electronic Materials; Sep2024, Vol. 53 Issue 9, p5062-5072, 11p
Publication Year :
2024

Abstract

Ca-doped BiFeO<subscript>3</subscript>/LaNiO<subscript>3</subscript>/LaAlO<subscript>3</subscript> (BCFO/LNO/LAO) heterostructures have garnered significant interest due to their unique combination of ferroelectric, magnetic, and resistive switching properties due to interfaces and lattice mismatch/strain, leading to unique electronic properties. The roles of structural defects and oxygen vacancies are important in achieving the magnetic and electrical properties of BiFeO<subscript>3</subscript>-based heterostructures. By generating defects, swift heavy ion irradiation can lead to changes in the structural, optical, electrical, and magnetic properties of the materials. The Ca-doped BiFeO<subscript>3</subscript> and LaNiO<subscript>3</subscript> heterostructure was grown upon LAO substrates using the pulsed laser deposition technique, ensuring high-quality interfaces and controlled thicknesses. The heterostructures were irradiated with 80 MeV O<superscript>+7</superscript> ions at various ion fluence levels (5 × 10<superscript>10</superscript> ions/cm<superscript>2</superscript> to 5 × 10<superscript>12</superscript> ions/cm<superscript>2</superscript>). The structure and crystalline orientation of the thin films were confirmed through x-ray diffraction, while the surface morphology was measured using atomic force microscopy. Irradiation-induced modifications of the structural strain and surface morphology were investigated in the context of internal annealing effect and defect formation. The resistive switching (RS) properties of the proposed devices were assessed by I–V measurement with sweeping 0 → 5 V → 0 → − 5 V → 0, which shows that irradiation-induced defects play an important role in the electrical properties of the proposed heterostructure. Bipolar RS behavior was also verified with the conduction mechanism, indicating that the ohmic and space-charge-limited conduction mechanism plays an important role in irradiated BCFO/LNO/LAO heterostructures. Graphical representation of the defect formation and RS behavior due to varying ion fluence as a function of RMS roughness and strain. [ABSTRACT FROM AUTHOR]

Details

Language :
English
ISSN :
03615235
Volume :
53
Issue :
9
Database :
Complementary Index
Journal :
Journal of Electronic Materials
Publication Type :
Academic Journal
Accession number :
178774746
Full Text :
https://doi.org/10.1007/s11664-024-11139-0