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Low-energy electronic structure in the unconventional charge-ordered state of ScV6Sn6.

Authors :
Kundu, Asish K.
Huang, Xiong
Seewald, Eric
Ritz, Ethan
Pakhira, Santanu
Zhang, Shuai
Sun, Dihao
Turkel, Simon
Shabani, Sara
Yilmaz, Turgut
Vescovo, Elio
Dean, Cory R.
Johnston, David C.
Valla, Tonica
Birol, Turan
Basov, Dmitri N.
Fernandes, Rafael M.
Pasupathy, Abhay N.
Source :
Nature Communications; 6/12/2024, Vol. 15 Issue 1, p1-9, 9p
Publication Year :
2024

Abstract

Kagome vanadates AV<subscript>3</subscript>Sb<subscript>5</subscript> display unusual low-temperature electronic properties including charge density waves (CDW), whose microscopic origin remains unsettled. Recently, CDW order has been discovered in a new material ScV<subscript>6</subscript>Sn<subscript>6</subscript>, providing an opportunity to explore whether the onset of CDW leads to unusual electronic properties. Here, we study this question using angle-resolved photoemission spectroscopy (ARPES) and scanning tunneling microscopy (STM). The ARPES measurements show minimal changes to the electronic structure after the onset of CDW. However, STM quasiparticle interference (QPI) measurements show strong dispersing features related to the CDW ordering vectors. A plausible explanation is the presence of a strong momentum-dependent scattering potential peaked at the CDW wavevector, associated with the existence of competing CDW instabilities. Our STM results further indicate that the bands most affected by the CDW are near vHS, analogous to the case of AV<subscript>3</subscript>Sb<subscript>5</subscript> despite very different CDW wavevectors. The authors use angle-resolved photoemission spectroscopy (ARPES) and scanning tunneling microscopy (STM) to study the charge density wave (CDW) in the kagome material ScV<subscript>6</subscript>Sn<subscript>6</subscript>. The ARPES data shows minimal changes to the electronic structure in the CDW state, while STM quasiparticle interference measurements imply a strong reconstruction of the electronic structure in the CDW state. [ABSTRACT FROM AUTHOR]

Details

Language :
English
ISSN :
20411723
Volume :
15
Issue :
1
Database :
Complementary Index
Journal :
Nature Communications
Publication Type :
Academic Journal
Accession number :
177881106
Full Text :
https://doi.org/10.1038/s41467-024-48883-0