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Quantifying CH4 emissions from coal mine aggregation areas in Shanxi, China, using TROPOMI observations and the wind-assigned anomaly method.

Authors :
Tu, Qiansi
Hase, Frank
Qin, Kai
Cohen, Jason Blake
Khosrawi, Farahnaz
Zou, Xinrui
Schneider, Matthias
Lu, Fan
Source :
Atmospheric Chemistry & Physics; 2024, Vol. 24 Issue 8, p4875-4894, 20p
Publication Year :
2024

Abstract

China stands out as a major contributor to anthropogenic methane (CH 4) emissions, with coal mine methane (CMM) playing a crucial role. To control and reduce CH 4 emissions, China has made a dedicated commitment and formulated an ambitious mitigation plan. To verify the progress made, the consistent acquisition of independent CH 4 emission data is required. This paper aims to implement a wind-assigned anomaly method for the precise determination of regional-scale CMM emissions within the coal-rich Shanxi province. We use the TROPOspheric Monitoring Instrument (TROPOMI) CH 4 observations from May 2018 to May 2023, coupled with ERA5 wind and a bottom-up inventory dataset based on the IPCC (Intergovernmental Panel on Climate Change) Tier 2 approach covering the Changzhi, Jincheng, and Yangquan regions of the Shanxi province. The derived emission strengths are 8.4 × 10 26 molec. s -1 (0.706 Tg yr -1 , ± 25 %), 1.4 × 10 27 molec. s -1 (1.176 Tg yr -1 , ± 20 %), and 4.9 × 10 26 molec. s -1 (0.412 Tg yr -1 , ± 21 %), respectively. Our results exhibit biases of - 18 %, 8 %, and 14 %, respectively, when compared to the IPCC Tier 2 bottom-up inventory. Larger discrepancies are found when comparing the estimates to the Copernicus Atmosphere Monitoring Service global anthropogenic emissions (CAMS-GLOB-ANT) and Emissions Database for Global Atmospheric Research (EDGARv7.0) inventories (64 %–176 %), suggesting that the two inventories may be overestimating CH 4 emissions from the studied coal mining regions. Our estimates provide a comprehensive characterization of the regions within the Shanxi province, contribute to the validation of emission inventories, and provide additional insights into CMM emission mitigation. [ABSTRACT FROM AUTHOR]

Details

Language :
English
ISSN :
16807316
Volume :
24
Issue :
8
Database :
Complementary Index
Journal :
Atmospheric Chemistry & Physics
Publication Type :
Academic Journal
Accession number :
177165453
Full Text :
https://doi.org/10.5194/acp-24-4875-2024