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Readily processed multifunctional SiC catalytic filter for industrial emissions control.

Authors :
Chen, Jiahao
Yin, Yongliang
Low, Ze‐Xian
Yuan, Kai
Wei, Wei
Zeng, Yiqing
Zhong, Zhaoxiang
Xing, Weihong
Source :
AIChE Journal; Apr2023, Vol. 69 Issue 4, p1-15, 15p
Publication Year :
2023

Abstract

One step fabrication of SiC catalytic filter is currently limited by the mismatched calcination temperature between SiC filter (>1700°C) and the catalysts (<800°C), and the difficulty in the chemical immobilization of catalysts. Here, a SrTi1−xCoxO3‐SiC (STC‐SiC) catalytic filter was directly fabricated from raw SiC grains and STC precursor oxides (SrCO3, TiO2, and Co3O4) via a single‐step reactive thermal processing (SRTP) approach, which significantly reduced energy consumption and sintering time over 50%. Acid etching enables the active TiO2 and Co3O4 nanoparticles spontaneously formed on STC catalysts in STC‐SiC catalytic filter (STC‐SiC‐A), which induces the generation of oxygen vacancies and facilitates the adsorption and activation of O2 and NO. The STC‐SiC‐A catalytic filter exhibits highly competitive NO oxidation of 60% and complete dust interception (100%) at 360°C. This work demonstrates an efficient and rapid processing technique of SiC based catalytic filters, which can also be implemented on other ceramic‐based catalytic filters. [ABSTRACT FROM AUTHOR]

Details

Language :
English
ISSN :
00011541
Volume :
69
Issue :
4
Database :
Complementary Index
Journal :
AIChE Journal
Publication Type :
Academic Journal
Accession number :
162595199
Full Text :
https://doi.org/10.1002/aic.17954