Spin-Filter Magnetic Tunnel Junctions Based on A-Type Antiferromagnetic CrSBr with Giant Tunnel Magnetoresistance.

CrSBr is a stable two-dimensional (2D) van der Waals (vdW) magnet with intralayer ferromagnetic and interlayer antiferromagnetic couplings. Here, we propose to use CrSBr as the barrier in spin-filter (sf) MTJ and establish the devices based on graphene/CrSBr/graphene structures. Employing density functional theory (DFT) combined with the nonequilibrium Green's function approach, we investigated the transmission details, and the results show TMR values above 330%, 2 × 10⁷% and 10⁵% with two-, four- and six-layer CrSBr at zero bias, respectively. Subsequently, we systematically analyze the transmission spectra, transmission eigenstates, electrostatic potentials, band structures and local density of states to elaborate the underlying mechanism of the TMR effect in the sf-MTJs. Our results indicate the great prospect of CrSBr-based sf-MTJs in applications, and provide guidance for futural experiments. [ABSTRACT FROM AUTHOR]