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Nonlinear electronic and ultrafast optical signatures in chemical vapor-deposited ultrathin PtS2 ribbons.
- Source :
- Nano Research; May2022, Vol. 15 Issue 5, p4366-4373, 8p
- Publication Year :
- 2022
-
Abstract
- The emerging two-dimensional (2D) platinum disulfide (PtS<subscript>2</subscript>) has driven increasing attentions due to its high electron mobility, good air-stability, and strong interlayer interaction which leads to a widely tunable electronic structure. However, a detailed study on its covalent-like layer-dependent properties remains infant. Herein, we demonstrate the successful production of ultrathin 1T-PtS<subscript>2</subscript> ribbons with thickness centralized almost at monolayer 1L–4L and large domain size up to 210 µm on Au foils using chemical vapor deposition (CVD) technique, which enables macro- and microscopic study of its extraordinary layer-dependent features with precise control of the number of layers. Using electron energy loss spectroscopy (EELS) and optical pump-probe spectroscopy (OPPS), we reveal that both the electron and ultrafast optical absorption signals of the as-grown 2D PtS<subscript>2</subscript> show strong nonlinear layer-dependent responses which manifest discriminated transition in 1L–4L PtS<subscript>2</subscript> ribbons. The layer-dependent nonlinear response of 2D PtS<subscript>2</subscript> can be well interpreted in the frame of calculated electron and phonon structures. These achievements offer a platform for successfully fabricating large-sized ultrathin 2D PtS<subscript>2</subscript> and facilitating our knowledge about its electronic and optoelectronic properties. [ABSTRACT FROM AUTHOR]
Details
- Language :
- English
- ISSN :
- 19980124
- Volume :
- 15
- Issue :
- 5
- Database :
- Complementary Index
- Journal :
- Nano Research
- Publication Type :
- Academic Journal
- Accession number :
- 156743136
- Full Text :
- https://doi.org/10.1007/s12274-022-4168-y