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Multidimensional spectroscopy of magneto-excitons at high magnetic fields.

Authors :
Mapara, V.
Stevens, C. E.
Paul, J.
Barua, A.
Reno, J. L.
McGill, S. A.
Hilton, D. J.
Karaiskaj, D.
Source :
Journal of Chemical Physics; 11/28/2021, Vol. 155 Issue 20, p1-10, 10p
Publication Year :
2021

Abstract

We perform two-dimensional Fourier transform spectroscopy on magneto-excitons in GaAs at magnetic fields and observe Zeeman splitting of the excitons. The Zeeman components are clearly resolved as separate peaks due to the two-dimensional nature of the spectra, leading to a more accurate measurement of the Zeeman splitting and the Landé g factors. Quantum coherent coupling between Zeeman components is observed using polarization dependent one-quantum two-dimensional spectroscopy. We use two-quantum two-dimensional spectroscopy to investigate higher four-particle correlations at high magnetic fields and reveal the role of the Zeeman splitting on the two-quantum transitions. The experimental two-dimensional spectra are simulated using the optical Bloch equations, where many-body effects are included phenomenologically. [ABSTRACT FROM AUTHOR]

Details

Language :
English
ISSN :
00219606
Volume :
155
Issue :
20
Database :
Complementary Index
Journal :
Journal of Chemical Physics
Publication Type :
Academic Journal
Accession number :
153907341
Full Text :
https://doi.org/10.1063/5.0070113