Challenging and Improving the Simulation of Mid‐Level Mixed‐Phase Clouds Over the High‐Latitude Southern Ocean.

Climate models exhibit major radiative biases over the Southern Ocean owing to a poor representation of mixed‐phase clouds. This study uses the remote‐sensing dataset from the Measurements of Aerosols, Radiation and Clouds over the Southern Ocean (MARCUS) campaign to assess the ability of the Weather Research and Forecasting (WRF) model to reproduce frontal clouds off Antarctica. It focuses on the modeling of thin mid‐level supercooled liquid water layers which precipitate ice. The standard version of WRF produces almost fully glaciated clouds and cannot reproduce cloud top turbulence. Our work demonstrates the importance of adapting the ice nucleation parameterization to the pristine austral atmosphere to reproduce the supercooled liquid layers. Once simulated, droplets significantly impact the cloud radiative effect by increasing downwelling longwave fluxes and decreasing downwelling shortwave fluxes at the surface. The net radiative effect is a warming of snow and ice covered surfaces and a cooling of the ocean. Despite improvements in our simulations, the local turbulent circulation related to cloud‐top radiative cooling is not properly reproduced, advocating for the need to develop a parameterization for top‐down convection to capture the turbulence‐microphysics interplay at cloud top. Plain Language Summary: Among the major shortcomings of climate models is a poor representation of clouds over the Southern Ocean. Thanks to new measurements from the Measurements of Aerosols, Radiation and Clouds over the Southern Ocean campaign that took place aboard the Aurora Australia ice breaker, we can now better assess the ability of models to represent clouds off Antarctica. In particular, we focus here on clouds that are mostly composed of ice crystals but that are topped by a thin layer of so‐called "supercooled" liquid droplets that form at temperatures below zero Celsius. While the standard version of the model produces clouds composed only of ice, we show that by adapting the formulation of ice crystal formation to the very pristine atmospheric conditions peculiar to the Southern Ocean it is possible to successfully reproduce thin layers of supercooled liquid droplets observed in mixed‐phase clouds. The latter significantly changes how much sunlight these clouds reflect to space, which is critical to understanding the climate. Compared to ice crystals, liquid droplets tend to reflect more solar energy toward space and at the same time, they enhance the cloud infrared emission toward the surface of the Antarctic ice sheet. Key Points: Weather Research and Forecasting‐observation comparison during Measurements of Aerosols, Radiation and Clouds over the Southern Ocean shows the inability of the model in standard configurations to simulate austral mixed‐phase cloudsA parameterization of ice nucleation based on new ice nucleating particle measurements improves the simulation of supercooled liquid water near cloud topFurther parameterization developments targeting the convection at cloud top are needed to reproduce the turbulence‐microphysics interplay [ABSTRACT FROM AUTHOR]