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2010-2015 North American methane emissions, sectoral contributions, and trends: a high-resolution inversion of GOSAT satellite observations of atmospheric methane.

Authors :
Maasakkers, Joannes D.
Jacob, Daniel J.
Sulprizio, Melissa P.
Scarpelli, Tia R.
Hannah Nesser
Jianxiong Sheng
Yuzhong Zhang
Xiao Lu
Bloom, A. Anthony
Bowman, Kevin W.
Worden, John R.
Parker, Robert J.
Source :
Atmospheric Chemistry & Physics Discussions; 9/18/2020, p1-28, 28p
Publication Year :
2020

Abstract

We use 2010-2015 GOSAT satellite observations of atmospheric methane columns over North America in a high-resolution inversion of methane emissions, including contributions from different sectors and long-term trends. The inversion involves analytical solution to the Bayesian optimization problem for a Gaussian mixture model (GMM) of the emission field with up to 0.5° x 0.625° resolution in concentrated source regions. Analytical solution provides a closed-form characterization of the information content from the inversion and facilitates the construction of a large ensemble of solutions exploring the effect of different uncertainties and assumptions. Prior estimates for the inversion include a gridded version of the EPA Inventory of U.S. Greenhouse Gas Emissions and Sinks (GHGI) and the WetCHARTS model ensemble for wetlands. Our best estimate for mean 2010-2015 US anthropogenic emissions is 30.6 (range: 29.4-31.3) Tg a<superscript>-1</superscript>, slightly higher than the gridded EPA inventory (28.7 (26.4-36.2) Tg a<superscript>-1</superscript>). The main discrepancy is for the oil and gas production sectors where we find higher emissions than the GHGI by 35 % and 22 % respectively. The most recent version of the EPA GHGI revises downward its estimate of emissions from oil production and we find that these are a factor 2 lower than our estimate. Our best estimate of US wetland emissions is 10.2 (5.6-11.1) Tg a<superscript>-1</superscript>, on the low end of the prior WetCHARTS inventory uncertainty range (14.2 (3.3-32.4) Tg a<superscript>-1</superscript>) and calling for better understanding of these emissions. We find an increasing trend in US anthropogenic emissions over 2010-2015 of 0.4 % a<superscript>-1</superscript>, lower than previous GOSAT-based estimates but opposite to the decrease reported by the EPA GHGI. Most of this increase appears driven by unconventional oil/gas production in the eastern US. We also find that oil/gas production emissions in Mexico are higher than in the nationally reported inventory, though there is evidence for a 2010-2015 decrease in emissions from offshore oil production. [ABSTRACT FROM AUTHOR]

Details

Language :
English
ISSN :
16807367
Database :
Complementary Index
Journal :
Atmospheric Chemistry & Physics Discussions
Publication Type :
Academic Journal
Accession number :
145928842
Full Text :
https://doi.org/10.5194/acp-2020-915