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Invited Article: High resolution angle resolved photoemission with tabletop 11 eV laser.

Authors :
Yu He
Vishik, Inna M.
Ming Yi
Shuolong Yang
Zhongkai Liu
Lee, James J.
Sudi Chen
Rebec, Slavko N.
Leuenberger, Dominik
Zong, Alfred
Jefferson, C. Michael
Moore, Robert G.
Kirchmann, Patrick S.
Merriam, Andrew J.
Zhi-Xun Shen
Source :
Review of Scientific Instruments; Jan2016, Vol. 87 Issue 1, p1-11, 11p, 2 Color Photographs, 2 Black and White Photographs, 1 Diagram, 1 Chart, 5 Graphs
Publication Year :
2016

Abstract

We developed a table-top vacuum ultraviolet (VUV) laser with 113 778 nm wavelength (10.897 eV) . and demonstrated its viability as a photon source for high resolution angle-resolved photoemission spectroscopy (ARPES). This sub-nanosecond pulsed VUV laser operates at a repetition rate of 10 MHz, provides a flux of 2 x 10<superscript>12</superscript> photons/s, and enables photoemission with energy and momentum resolutions better than 2 meV and 0.012 Å<superscript>-1</superscript>, respectively. Space-charge induced energy shifts and spectral broadenings can be reduced below 2 meV. The setup reaches electron momenta up to 1.2 Å<superscript>11</superscript>, granting full access to the first Brillouin zone of most materials. Control over the linear polarization, repetition rate, and photon flux of the VUV source facilitates ARPES investigations of a broad range of quantum materials, bridging the application gap between contemporary low energy laser-based ARPES and synchrotron-based ARPES. We describe the principles and operational characteristics of this source and showcase its performance for rare earth metal tritellurides, high temperature cuprate superconductors, and iron-based superconductors. [ABSTRACT FROM AUTHOR]

Details

Language :
English
ISSN :
00346748
Volume :
87
Issue :
1
Database :
Complementary Index
Journal :
Review of Scientific Instruments
Publication Type :
Academic Journal
Accession number :
112702489
Full Text :
https://doi.org/10.1063/1.4939759