Quantum Geometric Moment Encodes Stacking Order of Moiré Matter.

Exploring the topological characteristics of electronic bands is essential in condensed matter physics. Moiré materials featuring flat bands provide a versatile platform for engineering band topology and correlation effects. In moiré materials that break either time-reversal symmetry or inversion symmetry or both, electronic bands exhibit Berry curvature hotspots. Different stacking orders in these materials result in varied Berry curvature distributions within the flat bands, even when the band dispersion remains similar. However, experimental studies probing the impact of stacking order on the quantum geometric quantities are lacking. 1.4° twisted double bilayer graphene (TDBG) facilitates two distinct stacking orders (AB-AB, AB-BA) and forms an inversion broken moiré superlattice with electrically tunable flat bands. The valley Chern numbers of the flat bands depend on the stacking order, and the nonlinear Hall (NLH) effect distinguishes the differences in Berry curvature dipole (BCD), the first moment of Berry curvature. The BCD exhibits antisymmetric behavior, flipping its sign with the polarity of the perpendicular electric field in AB-AB TDBG, while it displays a symmetric behavior, maintaining the same sign regardless of the electric field's polarity in AB-BA TDBG. This approach electronically detects stacking-induced quantum geometry, while opening a pathway to quantum geometry engineering and detection.
(© 2025 The Author(s). Advanced Materials published by Wiley‐VCH GmbH.)