Back to Search Start Over

Topologically Engineered High- Q Quasi-BIC Metasurfaces for Enhanced Near-Infrared Emission in PbS Quantum Dots.

Authors :
Guo J
Jin R
Fu Z
Zhang Y
Yu F
Chen J
Wang X
Huang L
Zhou C
Chen X
Lu W
Li G
Source :
Nano letters [Nano Lett] 2025 Jan 15. Date of Electronic Publication: 2025 Jan 15.
Publication Year :
2025
Publisher :
Ahead of Print

Abstract

Enhancing photoluminescence (PL) efficiency in colloidal quantum dots is pivotal for next-generation near-infrared photodetectors, imaging systems, and photonic devices. Conventional methods, especially metal-based plasmonic structures, suffer from large optical losses, which limits their practical use. Here, we introduce a quasi-bound state in the continuum (quasi-BIC) metasurface on a silicon-on-insulator platform, tailored to provide high-quality factor resonances with minimized losses. Utilizing topological charge engineering and controlled in-plane asymmetry in silicon cylinder arrays, we developed a robust quasi-BIC capable of maintaining a high Q factor across a broad angular range, achieving an experimental Q factor of 3031 at normal incidence. This approach significantly enhances near-field interactions, achieving a ≤110-fold increase in PL for PbS quantum dots at 33 K and a 41-fold enhancement at room temperature. Our findings offer a scalable, cost-effective solution for enhancing light emission in advanced optoelectronic applications.

Details

Language :
English
ISSN :
1530-6992
Database :
MEDLINE
Journal :
Nano letters
Publication Type :
Academic Journal
Accession number :
39812516
Full Text :
https://doi.org/10.1021/acs.nanolett.4c05710