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Resonance-Amplified Terahertz Near-Field Spectroscopy of a Single Nanowire.

Authors :
Norman S
Chu G
Peng K
Seddon J
Hale LL
Tan HH
Jagadish C
Mouthaan R
Alexander-Webber J
Joyce HJ
Johnston MB
Mitrofanov O
Siday T
Source :
Nano letters [Nano Lett] 2024 Dec 11; Vol. 24 (49), pp. 15716-15723. Date of Electronic Publication: 2024 Nov 26.
Publication Year :
2024

Abstract

Nanoscale material systems are central to next-generation optoelectronic and quantum technologies, yet their development remains hindered by limited characterization tools, particularly at terahertz (THz) frequencies. Far-field THz spectroscopy techniques lack the sensitivity for investigating individual nanoscale systems, whereas in near-field THz nanoscopy, surface states, disorder, and sample-tip interactions often mask the response of the entire nanoscale system. Here, we present a THz resonance-amplified near-field spectroscopy technique that can detect subtle conductivity changes in isolated nanoscale systems─such as a single InAs nanowire─under ultrafast photoexcitation. By exploiting the spatial localization and resonant field enhancement in the gap of a bowtie antenna, our approach enables precise measurements of the nanostructures through shifts in the antenna resonant frequency, offering a direct means of extracting the system response, and unlocking investigations of ultrafast charge-carrier dynamics in isolated nanoscale and microscale systems.

Details

Language :
English
ISSN :
1530-6992
Volume :
24
Issue :
49
Database :
MEDLINE
Journal :
Nano letters
Publication Type :
Academic Journal
Accession number :
39588607
Full Text :
https://doi.org/10.1021/acs.nanolett.4c04395