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Experimental investigation of gamma-ray interaction parameters and buildup factors in lanthanide compounds: Insights into penetration depth.

Authors :
Manjunatha
Bennal AS
Hosamani MM
Hiremath GB
Singh VP
Badiger NM
Source :
Applied radiation and isotopes : including data, instrumentation and methods for use in agriculture, industry and medicine [Appl Radiat Isot] 2024 Oct; Vol. 212, pp. 111466. Date of Electronic Publication: 2024 Aug 03.
Publication Year :
2024

Abstract

This experimental investigation focuses on the gamma-ray interaction parameters and the buildup factor in lanthanide compounds (CeO <subscript>2</subscript> , Ce(SO <subscript>4</subscript> ) <subscript>2</subscript> , Dy <subscript>2</subscript> (SO <subscript>4</subscript> ) <subscript>3</subscript> , C <subscript>3</subscript> O <subscript>9</subscript> Sm <subscript>2</subscript> , C <subscript>3</subscript> Gd <subscript>2</subscript> O <subscript>9</subscript> , Pr <subscript>2</subscript> O <subscript>3</subscript> ). These compounds were exposed to weak radioactive gamma sources with energies of 356, 511, 662, 1173, 1275, and 1332 keV by adopting narrow and broad beam geometry experimental arrangements. The incident and transmitted radiation intensities were measured using a NaI (Tl) detector. Experimentally measured values of mass attenuation coefficient and effective atomic number of lanthanide compounds were found to be in precise agreement with theoretical values obtained from NIST XCOM and Direct-Z <subscript>eff</subscript> database respectively. Additionally, the experimentally determined buildup factor values were compared with energy absorption buildup factor (EABF) and exposure buildup factor (EBF) values obtained from Phy-X/PSD software, providing insights into the gamma-ray penetration depth in terms of mean free path (MFP). At 356 keV, the EABF analysis showed that most compounds had a penetration depth of around 8 mean free paths. In contrast, the EBF analysis indicated penetration depths exceeding 10 mean free paths for all compounds except Ce (SO <subscript>4</subscript> ) <subscript>2</subscript> . This new approach holds immense potential for transformative advancements in medical diagnostics, therapy, and the development of innovative technologies in nuclear sciences.<br />Competing Interests: Declaration of competing interest The authors declare the following financial interests/personal relationships which may be considered as potential competing interests: Aravind S. Bennal reports financial support was provided by University Grants Commission Department of Atomic Energy Consortium for Scientific Research. If there are other authors, they declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper.<br /> (Copyright © 2024 Elsevier Ltd. All rights reserved.)

Details

Language :
English
ISSN :
1872-9800
Volume :
212
Database :
MEDLINE
Journal :
Applied radiation and isotopes : including data, instrumentation and methods for use in agriculture, industry and medicine
Publication Type :
Academic Journal
Accession number :
39126755
Full Text :
https://doi.org/10.1016/j.apradiso.2024.111466