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Decarboxylative C-N Coupling of 2,2-Difluorobicyclo[1.1.1]pentane (BCP-F 2 ) Building Blocks.

Authors :
Ma X
Chen JL
Gaskins BE
Source :
Organic letters [Org Lett] 2024 Mar 08; Vol. 26 (9), pp. 1947-1951. Date of Electronic Publication: 2024 Feb 22.
Publication Year :
2024

Abstract

Described herein is our effort toward achieving the decarboxylative functionalization of 2,2-difluorobicyclo[1.1.1]pentane (BCP-F <subscript>2</subscript> ) building blocks. When compared with the nonfluorinated bicyclo[1.1.1]pentane (BCP) analogues, we discovered divergent reactivities. This is the first successful decarboxylative coupling of BCP-F <subscript>2</subscript> building blocks reported via the photoredox mechanism.

Details

Language :
English
ISSN :
1523-7052
Volume :
26
Issue :
9
Database :
MEDLINE
Journal :
Organic letters
Publication Type :
Academic Journal
Accession number :
38386927
Full Text :
https://doi.org/10.1021/acs.orglett.4c00307