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Tailoring ionomer distribution in the catalyst layer via heteroatom-functionalization toward superior PEMFC performance.

Authors :
Sun D
Zhao Z
Jin M
Zhang H
Source :
Chemical communications (Cambridge, England) [Chem Commun (Camb)] 2023 Sep 21; Vol. 59 (76), pp. 11357-11360. Date of Electronic Publication: 2023 Sep 21.
Publication Year :
2023

Abstract

We investigate in detail the influence of O, S, and N functionalization of Pt <subscript>3</subscript> Co/C catalysts on the proton exchange membrane fuel cell (PEMFC). The results demonstrated that N-functionalization is more beneficial for the distribution of the ionomer in the catalyst layer, resulting in a trade-off between oxygen and hydronium ion transport.

Details

Language :
English
ISSN :
1364-548X
Volume :
59
Issue :
76
Database :
MEDLINE
Journal :
Chemical communications (Cambridge, England)
Publication Type :
Academic Journal
Accession number :
37670613
Full Text :
https://doi.org/10.1039/d3cc03610c