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A modified magnetic bottle electron spectrometer for the detection of multiply charged ions in coincidence with all correlated electrons: decay pathways to Xe 3+ above xenon-4d ionization threshold.

Authors :
Ismail I
Khalal MA
Huttula M
Jänkälä K
Bizau JM
Cubaynes D
Hikosaka Y
Bučar K
Žitnik M
Andric L
Lablanquie P
Palaudoux J
Penent F
Source :
Physical chemistry chemical physics : PCCP [Phys Chem Chem Phys] 2022 Aug 31; Vol. 24 (34), pp. 20219-20227. Date of Electronic Publication: 2022 Aug 31.
Publication Year :
2022

Abstract

Single-photon multiple photoionization results from electron correlations that make this process possible beyond the independent electron approximation. To study this phenomenon experimentally, the detection in coincidence of all emitted electrons is the most direct approach. It provides the relative contribution of all possible multiple ionization processes, the energy distribution between electrons that can reveal simultaneous or sequential mechanisms, and, if possible, the angular correlations between electrons. In the present work, we present a new magnet design of our magnetic bottle electron spectrometer that allows the detection of multiply charged Xe <superscript> n +</superscript> ions in coincidence with n electrons. This new coincidence detection allows more efficient extraction of minor channels that are otherwise masked by random coincidences. The proof of principle is provided for xenon triple ionization.

Details

Language :
English
ISSN :
1463-9084
Volume :
24
Issue :
34
Database :
MEDLINE
Journal :
Physical chemistry chemical physics : PCCP
Publication Type :
Academic Journal
Accession number :
35983783
Full Text :
https://doi.org/10.1039/d2cp02930h