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Directional Laser from Solution-Grown Grating-Patterned Perovskite Single-Crystal Microdisks.
- Source :
-
Angewandte Chemie (International ed. in English) [Angew Chem Int Ed Engl] 2022 Aug 22; Vol. 61 (34), pp. e202205636. Date of Electronic Publication: 2022 Jul 08. - Publication Year :
- 2022
-
Abstract
- Solution-processed, high-gain, and wavelength-tunable perovskite single-crystal microdisk (PVKsc-MD) lasers have emerged as prospective coherent light sources in advanced nanophotonic designs. However, the inevitable multi-directional emission from a highly symmetrical cavity leads to low light collection efficiency which greatly hinders its application in integrated optical circuits. Here, we report on surface-patterned MAPbBr <subscript>3</subscript> PVKsc-MDs synthesized by a cost-efficient bottom-up solution process employing spin-coating and confined-growth nanoimprinting. The patterned microdisks have high crystal quality with regular shape and sharp edges and nano-grating structure on the upper surface. This straightforward process yields surface-patterned PVKsc-MD lasers with a low lasing threshold and high quality (Q) factor. In addition, the grating structure patterned on the PVKsc-MDs reduces the original symmetry of the laser cavity, which improves the emission directionality four times.<br /> (© 2022 Wiley-VCH GmbH.)
Details
- Language :
- English
- ISSN :
- 1521-3773
- Volume :
- 61
- Issue :
- 34
- Database :
- MEDLINE
- Journal :
- Angewandte Chemie (International ed. in English)
- Publication Type :
- Academic Journal
- Accession number :
- 35698256
- Full Text :
- https://doi.org/10.1002/anie.202205636