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Monthly Global Estimates of Fine Particulate Matter and Their Uncertainty.

Authors :
van Donkelaar A
Hammer MS
Bindle L
Brauer M
Brook JR
Garay MJ
Hsu NC
Kalashnikova OV
Kahn RA
Lee C
Levy RC
Lyapustin A
Sayer AM
Martin RV
Source :
Environmental science & technology [Environ Sci Technol] 2021 Nov 16; Vol. 55 (22), pp. 15287-15300. Date of Electronic Publication: 2021 Nov 01.
Publication Year :
2021

Abstract

Annual global satellite-based estimates of fine particulate matter (PM <subscript>2.5</subscript> ) are widely relied upon for air-quality assessment. Here, we develop and apply a methodology for monthly estimates and uncertainties during the period 1998-2019, which combines satellite retrievals of aerosol optical depth, chemical transport modeling, and ground-based measurements to allow for the characterization of seasonal and episodic exposure, as well as aid air-quality management. Many densely populated regions have their highest PM <subscript>2.5</subscript> concentrations in winter, exceeding summertime concentrations by factors of 1.5-3.0 over Eastern Europe, Western Europe, South Asia, and East Asia. In South Asia, in January, regional population-weighted monthly mean PM <subscript>2.5</subscript> concentrations exceed 90 μg/m <superscript>3</superscript> , with local concentrations of approximately 200 μg/m <superscript>3</superscript> for parts of the Indo-Gangetic Plain. In East Asia, monthly mean PM <subscript>2.5</subscript> concentrations have decreased over the period 2010-2019 by 1.6-2.6 μg/m <superscript>3</superscript> /year, with decreases beginning 2-3 years earlier in summer than in winter. We find evidence that global-monitored locations tend to be in cleaner regions than global mean PM <subscript>2.5</subscript> exposure, with large measurement gaps in the Global South. Uncertainty estimates exhibit regional consistency with observed differences between ground-based and satellite-derived PM <subscript>2.5</subscript> . The evaluation of uncertainty for agglomerated values indicates that hybrid PM <subscript>2.5</subscript> estimates provide precise regional-scale representation, with residual uncertainty inversely proportional to the sample size.

Details

Language :
English
ISSN :
1520-5851
Volume :
55
Issue :
22
Database :
MEDLINE
Journal :
Environmental science & technology
Publication Type :
Academic Journal
Accession number :
34724610
Full Text :
https://doi.org/10.1021/acs.est.1c05309