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UV-assisted ultrafast construction of robust Fe 3 O 4 /polydopamine/Ag Fenton-like catalysts for highly efficient micropollutant decomposition.

Authors :
Cheng S
Pan X
Zhang C
Lin X
Zhuang Q
Jiao Y
Dong W
Qi X
Source :
The Science of the total environment [Sci Total Environ] 2022 Mar 01; Vol. 810, pp. 151182. Date of Electronic Publication: 2021 Oct 26.
Publication Year :
2022

Abstract

Fenton-like catalysts represent a family of promising materials to degrade micropollutants from contaminated water. However, the practical applications of Fenton-like catalysts are mainly limited by low catalytic degradation efficiency and stability. Herein, for the first time, rapid fabrication of Ag-decorated Fe <subscript>3</subscript> O <subscript>4</subscript> /polydopamine (FPA) microspheres was achieved via the help of UV irradiation, and the designed FPA microspheres were employed as Fenton-like catalysts to degrade micropollutants. Results showed that UV irradiation could activate the generation of the polydopamine shell and accelerate the Ag deposition, which played a crucial role in the rapid synthesis of highly active and stable FPA catalysts. Relative to reported catalysts, these FPA microspheres exhibited outstanding catalytic degradation performance, achieving 94.38% removal of tetracycline within 60 min. This work will provide a convenient strategy in the sustainable and efficient purification of wastewater to improve the quality of human life.<br />Competing Interests: Declaration of competing interest The authors declare no conflict of interest.<br /> (Copyright © 2021 Elsevier B.V. All rights reserved.)

Details

Language :
English
ISSN :
1879-1026
Volume :
810
Database :
MEDLINE
Journal :
The Science of the total environment
Publication Type :
Academic Journal
Accession number :
34710406
Full Text :
https://doi.org/10.1016/j.scitotenv.2021.151182