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Europe-Wide Atmospheric Radionuclide Dispersion by Unprecedented Wildfires in the Chernobyl Exclusion Zone, April 2020.

Authors :
Masson O
Romanenko O
Saunier O
Kirieiev S
Protsak V
Laptev G
Voitsekhovych O
Durand V
Coppin F
Steinhauser G
de Vismes Ott A
Renaud P
Didier D
Boulet B
Morin M
Hýža M
Camps J
Belyaeva O
Dalheimer A
Eleftheriadis K
Gascó-Leonarte C
Ioannidou A
Isajenko K
Karhunen T
Kastlander J
Katzlberger C
Kierepko R
Knetsch GJ
Kónyi JK
Mietelski JW
Mirsch M
Møller B
Nikolić JK
Povinec PP
Rusconi R
Samsonov V
Sýkora I
Simion E
Steinmann P
Stoulos S
Suarez-Navarro JA
Wershofen H
Zapata-García D
Zorko B
Source :
Environmental science & technology [Environ Sci Technol] 2021 Oct 19; Vol. 55 (20), pp. 13834-13848. Date of Electronic Publication: 2021 Sep 29.
Publication Year :
2021

Abstract

From early April 2020, wildfires raged in the highly contaminated areas around the Chernobyl nuclear power plant (CNPP), Ukraine. For about 4 weeks, the fires spread around and into the Chernobyl exclusion zone (CEZ) and came within a few kilometers of both the CNPP and radioactive waste storage facilities. Wildfires occurred on several occasions throughout the month of April. They were extinguished, but weather conditions and the spread of fires by airborne embers and smoldering fires led to new fires starting at different locations of the CEZ. The forest fires were only completely under control at the beginning of May, thanks to the tireless and incessant work of the firefighters and a period of sustained precipitation. In total, 0.7-1.2 TBq <superscript>137</superscript> Cs were released into the atmosphere. Smoke plumes partly spread south and west and contributed to the detection of airborne <superscript>137</superscript> Cs over the Ukrainian territory and as far away as Western Europe. The increase in airborne <superscript>137</superscript> Cs ranged from several hundred μBq·m <superscript>-3</superscript> in northern Ukraine to trace levels of a few μBq·m <superscript>-3</superscript> or even within the usual background level in other European countries. Dispersion modeling determined the plume arrival time and was helpful in the assessment of the possible increase in airborne <superscript>137</superscript> Cs concentrations in Europe. Detections of airborne <superscript>90</superscript> Sr (emission estimate 345-612 GBq) and Pu (up to 75 GBq, mostly <superscript>241</superscript> Pu) were reported from the CEZ. Americium-241 represented only 1.4% of the total source term corresponding to the studied anthropogenic radionuclides but would have contributed up to 80% of the inhalation dose.

Details

Language :
English
ISSN :
1520-5851
Volume :
55
Issue :
20
Database :
MEDLINE
Journal :
Environmental science & technology
Publication Type :
Academic Journal
Accession number :
34585576
Full Text :
https://doi.org/10.1021/acs.est.1c03314