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Imaging the coherent propagation of collective modes in the excitonic insulator Ta 2 NiSe 5 at room temperature.

Authors :
Bretscher HM
Andrich P
Murakami Y
Golež D
Remez B
Telang P
Singh A
Harnagea L
Cooper NR
Millis AJ
Werner P
Sood AK
Rao A
Source :
Science advances [Sci Adv] 2021 Jul 07; Vol. 7 (28). Date of Electronic Publication: 2021 Jul 07 (Print Publication: 2021).
Publication Year :
2021

Abstract

Excitonic insulators host a condensate of electron-hole pairs at equilibrium, giving rise to collective many-body effects. Although several materials have emerged as excitonic insulator candidates, evidence of long-range coherence is lacking and the origin of the ordered phase in these systems remains controversial. Here, using ultrafast pump-probe microscopy, we investigate the possible excitonic insulator Ta <subscript>2</subscript> NiSe <subscript>5</subscript> Below 328 K, we observe the anomalous micrometer-scale propagation of coherent modes at velocities of ~10 <superscript>5</superscript> m/s, which we attribute to the hybridization between phonon modes and the phase mode of the condensate. We develop a theoretical framework to support this explanation and propose that electronic interactions provide a substantial contribution to the ordered phase in Ta <subscript>2</subscript> NiSe <subscript>5</subscript> These results allow us to understand how the condensate's collective modes transport energy and interact with other degrees of freedom. Our study provides a unique paradigm for the investigation and manipulation of these properties in strongly correlated materials.<br /> (Copyright © 2021 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution License 4.0 (CC BY).)

Details

Language :
English
ISSN :
2375-2548
Volume :
7
Issue :
28
Database :
MEDLINE
Journal :
Science advances
Publication Type :
Academic Journal
Accession number :
34233871
Full Text :
https://doi.org/10.1126/sciadv.abd6147