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Inorganic Perovskite Quantum Dot-Based Strain Sensors for Data Storage and In-Sensor Computing.

Authors :
Li MZ
Guo LC
Ding GL
Zhou K
Xiong ZY
Han ST
Zhou Y
Source :
ACS applied materials & interfaces [ACS Appl Mater Interfaces] 2021 Jul 07; Vol. 13 (26), pp. 30861-30873. Date of Electronic Publication: 2021 Jun 24.
Publication Year :
2021

Abstract

Although remarkable improvement has been achieved in stretchable strain sensors, challenges still exist in aspects including intelligent sensing, simultaneous data processing, and scalable fabrication techniques. In this work, a strain-sensitive device is presented by fabricating a CsPbBr <subscript>3</subscript> quantum dots (QDs) floating-gate field-effect transistor (FET) sensing array on thin polyimide (PI) films. The FET exhibits an excellent on/off ratio (>10 <superscript>3</superscript> ) and a large memory window (>2 V). With the introduction of CsPbBr <subscript>3</subscript> QDs as the trapping layer, an additional UV response is obtained because of the photogenerated charge carriers that significantly enhance the source-drain current ( I <subscript>DS</subscript> ) of the device. At each electrical state, the I <subscript>DS</subscript> varies with the strains and the sensing range is from compressive +12.5% to tensile -10.8%. Excellent data retainability and mechanical durability demonstrate the high quality and reliability of the fabricated sensors. Furthermore, synapse functions including long-term potentiation (LTP), long-term depression (LTD), etc., are emulated at the device level. Linearity factor changes of LTP/LTD in different sensing scenarios demonstrate the reliability of the device and further confirm the different sensing mechanisms with/without UV illumination. Our results exhibit the potential of transistor-based devices for multifunctional intelligent sensing.

Details

Language :
English
ISSN :
1944-8252
Volume :
13
Issue :
26
Database :
MEDLINE
Journal :
ACS applied materials & interfaces
Publication Type :
Academic Journal
Accession number :
34164986
Full Text :
https://doi.org/10.1021/acsami.1c07928