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Atom-surface van der Waals potentials of topological insulators and semimetals from scattering measurements.

Authors :
Tamtögl A
Ruckhofer A
Campi D
Allison W
Ernst WE
Source :
Physical chemistry chemical physics : PCCP [Phys Chem Chem Phys] 2021 Apr 07; Vol. 23 (13), pp. 7637-7652. Date of Electronic Publication: 2021 Jan 25.
Publication Year :
2021

Abstract

The phenomenology of resonant scattering has been known since the earliest experiments upon scattering of atomic beams from surfaces and is a means of obtaining experimental information about the fundamentals of weak adsorption systems in the van der Waals regime. We provide an overview of the experimental approach based on new experimental data for the He-Sb <subscript>2</subscript> Te <subscript>3</subscript> (111) system, followed by a comparative overview and perspective of recent results for topological semimetal and insulator surfaces. Moreover, we shortly discuss the perspectives of calculating helium-surface interaction potentials from ab initio calculations. Our perspective demonstrates that atom-surface scattering provides direct experimental information about the atom-surface interaction in the weak physisorption regime and can also be used to determine the lifetime and mean free path of the trapped atom. We further discuss the effects of elastic and inelastic scattering on the linewidth and lifetime of the trapped He atom with an outlook on future developments and applications.

Details

Language :
English
ISSN :
1463-9084
Volume :
23
Issue :
13
Database :
MEDLINE
Journal :
Physical chemistry chemical physics : PCCP
Publication Type :
Academic Journal
Accession number :
33492313
Full Text :
https://doi.org/10.1039/d0cp05388k