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Room-Temperature Electron-Hole Liquid in Monolayer MoS 2 .

Authors :
Yu Y
Bataller AW
Younts R
Yu Y
Li G
Puretzky AA
Geohegan DB
Gundogdu K
Cao L
Source :
ACS nano [ACS Nano] 2019 Sep 24; Vol. 13 (9), pp. 10351-10358. Date of Electronic Publication: 2019 Sep 09.
Publication Year :
2019

Abstract

Excitons in semiconductors are usually noninteracting and behave like an ideal gas, but may condense to a strongly correlated liquid-like state, i . e ., electron-hole liquid (EHL), at high density and appropriate temperature. An EHL is a macroscopic quantum state with exotic properties and represents the ultimate attainable charge excitation density in steady states. It bears great promise for a variety of fields such as ultra-high-power photonics and quantum science and technology. However, the condensation of gas-like excitons to an EHL has often been restricted to cryogenic temperatures, which significantly limits the prospect of EHLs for use in practical applications. Herein we demonstrate the formation of an EHL at room temperature in monolayer MoS <subscript>2</subscript> by taking advantage of the monolayer's extraordinarily strong exciton binding energy. This work demonstrates the potential for the liquid-like state of charge excitations to be a useful platform for the studies of macroscopic quantum phenomena and the development of optoelectronic devices.

Details

Language :
English
ISSN :
1936-086X
Volume :
13
Issue :
9
Database :
MEDLINE
Journal :
ACS nano
Publication Type :
Academic Journal
Accession number :
31483608
Full Text :
https://doi.org/10.1021/acsnano.9b04124