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Visible-Light Induction/Brønsted Acid Catalysis in Relay for the Enantioselective Synthesis of Tetrahydroquinolines.

Authors :
Xiong W
Li S
Fu B
Wang J
Wang QA
Yang W
Source :
Organic letters [Org Lett] 2019 Jun 07; Vol. 21 (11), pp. 4173-4176. Date of Electronic Publication: 2019 May 24.
Publication Year :
2019

Abstract

An efficient method merging Brønsted acid catalysis with visible-light induction for the highly enantioselective synthesis of tetrahydroquinolines has been developed. This mild process directly transforms 2-aminoenones into 2-substituted tetrahydroquinolines with excellent enantioselectivities through a relay visible-light-induced cyclization/chiral phosphoric acid-catalyzed transfer hydrogenation reaction.

Details

Language :
English
ISSN :
1523-7052
Volume :
21
Issue :
11
Database :
MEDLINE
Journal :
Organic letters
Publication Type :
Academic Journal
Accession number :
31124682
Full Text :
https://doi.org/10.1021/acs.orglett.9b01354