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Exploiting Boron Coordination: B←N Bond Supports a [2+2] Photodimerization in the Solid State and Generation of a Diboron Bis-Tweezer for Benzene/Thiophene Separation.

Authors :
Campillo-Alvarado G
D'mello KP
Swenson DC
Santhana Mariappan SV
Höpfl H
Morales-Rojas H
MacGillivray LR
Source :
Angewandte Chemie (International ed. in English) [Angew Chem Int Ed Engl] 2019 Apr 08; Vol. 58 (16), pp. 5413-5416. Date of Electronic Publication: 2019 Mar 12.
Publication Year :
2019

Abstract

B←N coordination supports a [2+2] photodimerization in the solid state. The bond is defined by an orthogonal interaction between stilbazole and a phenylboronic ester to enable a stereocontrolled and rapid photoreaction. The cyclobutane photoproduct affords a novel diboron bis-tweezer adduct that is used to separate a mixture of benzene and thiophene upon crystallization.<br /> (© 2019 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim.)

Details

Language :
English
ISSN :
1521-3773
Volume :
58
Issue :
16
Database :
MEDLINE
Journal :
Angewandte Chemie (International ed. in English)
Publication Type :
Academic Journal
Accession number :
30770618
Full Text :
https://doi.org/10.1002/anie.201812174