Back to Search Start Over

Assembly of the Entire Carbon Backbone of a Stereoisomer of the Antitumor Marine Natural Product Hemicalide.

Authors :
Lecourt C
Dhambri S
Yamani K
Boissonnat G
Specklin S
Fleury E
Hammad K
Auclair E
Sablé S
Grondin A
Arimondo PB
Sautel F
Massiot G
Meyer C
Cossy J
Sorin G
Lannou MI
Ardisson J
Source :
Chemistry (Weinheim an der Bergstrasse, Germany) [Chemistry] 2019 Feb 21; Vol. 25 (11), pp. 2745-2749. Date of Electronic Publication: 2019 Jan 25.
Publication Year :
2019

Abstract

A strategy for the assembly of the entire carbon backbone of a stereoisomer of the antitumor marine natural product hemicalide has been investigated. The devised convergent approach relies on Horner-Wadsworth-Emmons and Julia-Kocienski olefination reactions for the construction of the C6=C7 and C34=C35 double bonds, respectively, an aldol reaction to create the C27-C28 bond, and a Suzuki-Miyaura cross-coupling as the endgame to form the C15-C16 bond.<br /> (© 2019 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim.)

Details

Language :
English
ISSN :
1521-3765
Volume :
25
Issue :
11
Database :
MEDLINE
Journal :
Chemistry (Weinheim an der Bergstrasse, Germany)
Publication Type :
Academic Journal
Accession number :
30600846
Full Text :
https://doi.org/10.1002/chem.201806327