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[Composition Characteristics and Sources Apportionment of Lanthanoid in PM 2.5 of Quanzhou].

Authors :
Zhang YF
Yu RL
Hu GR
Sun JW
Xu WZ
Zhang ZW
Source :
Huan jing ke xue= Huanjing kexue [Huan Jing Ke Xue] 2017 Jul 08; Vol. 38 (7), pp. 2698-2706.
Publication Year :
2017

Abstract

Samples of PM <subscript>2.5</subscript> were collected from 5 sites in Quanzhou in March, April and July, 2014. The concentrations of lanthanoid and other trace metals in the PM <subscript>2.5</subscript> were determined by Inductively Coupled Plasma Mass Spectrometry(ICP-MS). The total lanthanoid concentration (Σ Loid ), the ratio of light-lanthanoid(L Loid, including, La, Ce, Pr, Nd, Sm and Eu) to heavy-lanthanoid(H Loid, including Gd, Tb, Dy, Ho, Er, Tm, Yb and Lu) in PM <subscript>2.5</subscript> were 2.490-5.708 ng·m <superscript>-3</superscript> (65.682-126.529 μg·g <superscript>-1</superscript> ) and 12.086-14.319, respectively. The distribution pattern of Loid in PM <subscript>2.5</subscript> was also evaluated in this study. All PM <subscript>2.5</subscript> samples showed similar distribution pattern with local topsoil. And positive Ce and negative Eu anomalies were observed in PM <subscript>2.5</subscript> . La-Ce-V plots and chemical mass balance(CMB) model were used for source identification and apportionment of PM <subscript>2.5</subscript> in Quanzhou. The CMB model was used to identify four main sources:urban fugitive dust, coal combustion, vehicle exhaust and waste incineration emission which had a contribution of 18.9%, 10.9%, 30.6% and 30.2%, respectively.

Details

Language :
Chinese
ISSN :
0250-3301
Volume :
38
Issue :
7
Database :
MEDLINE
Journal :
Huan jing ke xue= Huanjing kexue
Publication Type :
Academic Journal
Accession number :
29964608
Full Text :
https://doi.org/10.13227/j.hjkx.201612105