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In situ plasma-assisted atmospheric nitrogen fixation using water and spray-type jet plasma.

Authors :
Peng P
Chen P
Addy M
Cheng Y
Zhang Y
Anderson E
Zhou N
Schiappacasse C
Hatzenbeller R
Fan L
Liu S
Chen D
Liu J
Liu Y
Ruan R
Source :
Chemical communications (Cambridge, England) [Chem Commun (Camb)] 2018 Mar 15; Vol. 54 (23), pp. 2886-2889.
Publication Year :
2018

Abstract

In this study, a sustainable nitrogen fixation process was presented under atmospheric conditions and without introducing hydrogen or any catalyst. The novel in situ synthesis in this study used an advanced spray-type jet plasma, which significantly improved the fixation rate of nitrite, nitrate, and ammonium. Furthermore, the mechanism focusing on the co-synthesis of the abovementioned three nitrogen compounds was proposed based on the synergistic interactions between the gas-phase plasma and liquid surface dissociation.

Details

Language :
English
ISSN :
1364-548X
Volume :
54
Issue :
23
Database :
MEDLINE
Journal :
Chemical communications (Cambridge, England)
Publication Type :
Academic Journal
Accession number :
29497719
Full Text :
https://doi.org/10.1039/c8cc00697k