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Probing the Peroxycarbenium [3+2] Cycloaddition Reactions with 1,2-Disubstituted Ethylenes: Results and Insights.

Authors :
Xu ZJ
Wittlin S
Wu Y
Source :
Chemistry (Weinheim an der Bergstrasse, Germany) [Chemistry] 2017 Feb 10; Vol. 23 (9), pp. 2031-2034. Date of Electronic Publication: 2017 Jan 20.
Publication Year :
2017

Abstract

The causes for the title reaction to be limited to only the alkenes with an unsubstituted terminal alkenic carbon were explored. In some "failed" cases the cycloaddition products actually formed but rearranged concurrently. An oxygen atom or a N-Boc (Boc=tert-butyloxycarbonyl) group at the double bond was proven essential for acquisition of intact [3+2] cycloaddition products from 1,2-disubstituted ethylenes.<br /> (© 2017 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim.)

Details

Language :
English
ISSN :
1521-3765
Volume :
23
Issue :
9
Database :
MEDLINE
Journal :
Chemistry (Weinheim an der Bergstrasse, Germany)
Publication Type :
Academic Journal
Accession number :
28012253
Full Text :
https://doi.org/10.1002/chem.201605871