Back to Search Start Over

Selective Synthesis of Six Products from a Single Indolyl α-Diazocarbonyl Precursor.

Authors :
James MJ
O'Brien P
Taylor RJ
Unsworth WP
Source :
Angewandte Chemie (International ed. in English) [Angew Chem Int Ed Engl] 2016 Aug 08; Vol. 55 (33), pp. 9671-5. Date of Electronic Publication: 2016 Jul 20.
Publication Year :
2016

Abstract

Indolyl α-diazocarbonyls can be selectively cyclized to give six distinct products through the careful choice of catalyst and reaction conditions. A range of catalysts were used, including complexes of Rh(II) , Pd(II) , and Cu(II) , as well as SiO2 , to promote diazo decomposition and subsequent cyclization/rearrangement through a range of mechanistic pathways.<br /> (© 2016 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.)

Details

Language :
English
ISSN :
1521-3773
Volume :
55
Issue :
33
Database :
MEDLINE
Journal :
Angewandte Chemie (International ed. in English)
Publication Type :
Academic Journal
Accession number :
27435296
Full Text :
https://doi.org/10.1002/anie.201605337