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Synthesis of bench-stable diarylmethylium tetrafluoroborates.

Authors :
Barbero M
Buscaino R
Cadamuro S
Dughera S
Gualandi A
Marabello D
Cozzi PG
Source :
The Journal of organic chemistry [J Org Chem] 2015 May 01; Vol. 80 (9), pp. 4791-6. Date of Electronic Publication: 2015 Apr 23.
Publication Year :
2015

Abstract

A representative number of bench-stable nonsymmetric diarylcarbenium tetrafluoroborates have been isolated via the direct coupling of aryl (or heteroaryl) aldehydes and N-heteroarenes and fully characterized. They have proven to be highly stable in the presence of both EDG and EWG substituents. An (E)-iminium vinylogous substructure has been shown as the common cation scaffold by X-ray analysis and by NOE determination.

Details

Language :
English
ISSN :
1520-6904
Volume :
80
Issue :
9
Database :
MEDLINE
Journal :
The Journal of organic chemistry
Publication Type :
Academic Journal
Accession number :
25867788
Full Text :
https://doi.org/10.1021/acs.joc.5b00418