Back to Search Start Over

Lead halide perovskite nanowire lasers with low lasing thresholds and high quality factors.

Authors :
Zhu H
Fu Y
Meng F
Wu X
Gong Z
Ding Q
Gustafsson MV
Trinh MT
Jin S
Zhu XY
Source :
Nature materials [Nat Mater] 2015 Jun; Vol. 14 (6), pp. 636-42. Date of Electronic Publication: 2015 Apr 13.
Publication Year :
2015

Abstract

The remarkable performance of lead halide perovskites in solar cells can be attributed to the long carrier lifetimes and low non-radiative recombination rates, the same physical properties that are ideal for semiconductor lasers. Here, we show room-temperature and wavelength-tunable lasing from single-crystal lead halide perovskite nanowires with very low lasing thresholds (220 nJ cm(-2)) and high quality factors (Q ∼ 3,600). The lasing threshold corresponds to a charge carrier density as low as 1.5 × 10(16) cm(-3). Kinetic analysis based on time-resolved fluorescence reveals little charge carrier trapping in these single-crystal nanowires and gives estimated lasing quantum yields approaching 100%. Such lasing performance, coupled with the facile solution growth of single-crystal nanowires and the broad stoichiometry-dependent tunability of emission colour, makes lead halide perovskites ideal materials for the development of nanophotonics, in parallel with the rapid development in photovoltaics from the same materials.

Details

Language :
English
ISSN :
1476-4660
Volume :
14
Issue :
6
Database :
MEDLINE
Journal :
Nature materials
Publication Type :
Academic Journal
Accession number :
25849532
Full Text :
https://doi.org/10.1038/nmat4271