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Direct catalytic enantio- and diastereoselective ketone aldol reactions of isocyanoacetates.

Authors :
de la Campa R
Ortín I
Dixon DJ
Source :
Angewandte Chemie (International ed. in English) [Angew Chem Int Ed Engl] 2015 Apr 13; Vol. 54 (16), pp. 4895-8. Date of Electronic Publication: 2015 Mar 03.
Publication Year :
2015

Abstract

A catalytic asymmetric aldol addition/cyclization reaction of unactivated ketones with isocyanoacetate pronucleophiles has been developed. A quinine-derived aminophosphine precatalyst and silver oxide were found to be an effective binary catalyst system and promoted the reaction to afford chiral oxazolines possessing a fully substituted stereocenter with good diastereoselectivities and excellent enantioselectivities.<br /> (© 2015 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.)

Details

Language :
English
ISSN :
1521-3773
Volume :
54
Issue :
16
Database :
MEDLINE
Journal :
Angewandte Chemie (International ed. in English)
Publication Type :
Academic Journal
Accession number :
25735645
Full Text :
https://doi.org/10.1002/anie.201411852