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Strong 31P nuclear spin hyperpolarization produced via reversible chemical interaction with parahydrogen.

Authors :
Zhivonitko VV
Skovpin IV
Koptyug IV
Source :
Chemical communications (Cambridge, England) [Chem Commun (Camb)] 2015 Feb 14; Vol. 51 (13), pp. 2506-9.
Publication Year :
2015

Abstract

Substantial (31)P NMR signal enhancement of more than two orders of magnitude at 7 T for free and bound PPh3 species was observed under reversible interaction of (PPh3)3Ir(H2)Cl with parahydrogen. The large improvement in sensitivity made single-shot (31)P NMR imaging of a model object possible. The observed effects are temperature and magnetic field dependent as shown experimentally and theoretically.

Details

Language :
English
ISSN :
1364-548X
Volume :
51
Issue :
13
Database :
MEDLINE
Journal :
Chemical communications (Cambridge, England)
Publication Type :
Academic Journal
Accession number :
25358646
Full Text :
https://doi.org/10.1039/c4cc08115c