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Dearomatization strategy of β-enamino ester: construction of indenoazepines via tandem Michael addition/polycyclization.

Authors :
Yang M
Tang J
Fan R
Source :
Organic letters [Org Lett] 2013 Jul 05; Vol. 15 (13), pp. 3464-7. Date of Electronic Publication: 2013 Jun 24.
Publication Year :
2013

Abstract

A dearomatization strategy of β-enamino esters was developed to construct indenoazepine derivatives. The oxidative dearomatization was combined with a base-promoted tandem Michael addition/polycyclization and an acid-catalyzed aromatization. The nonaromatic structure of the Michael adducts might be essential to the realization of the 7-endo-dig cyclization.

Details

Language :
English
ISSN :
1523-7052
Volume :
15
Issue :
13
Database :
MEDLINE
Journal :
Organic letters
Publication Type :
Academic Journal
Accession number :
23795890
Full Text :
https://doi.org/10.1021/ol401553n