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Multi-particle collision dynamics simulations of sedimenting colloidal dispersions in confinement.

Authors :
Wysocki A
Royall CP
Winkler RG
Gompper G
Tanaka H
van Blaaderen A
Löwen H
Source :
Faraday discussions [Faraday Discuss] 2010; Vol. 144, pp. 245-52; discussion 323-45, 467-81.
Publication Year :
2010

Abstract

The sedimentation of an initially inhomogeneous distribution of hard-sphere colloids confined in a slit is simulated using the multi-particle collision dynamics scheme which takes into account hydrodynamic interactions mediated by the solvent. This system is an example for soft matter driven out of equilibrium where various length and time scales are involved. The initial laterally homogeneous density profiles exhibit a hydrodynamic Rayleigh-Taylor-like instability. Solvent backflow effects lead to an intricate non-linear behaviour which is analyzed via the solvent flow field and the colloidal velocity correlation function. Our simulation data are in good agreement with real-space microscopy experiments.

Details

Language :
English
ISSN :
1359-6640
Volume :
144
Database :
MEDLINE
Journal :
Faraday discussions
Publication Type :
Academic Journal
Accession number :
20158032
Full Text :
https://doi.org/10.1039/b901640f