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Discovery of potent furan piperazine sodium channel blockers for treatment of neuropathic pain.

Authors :
Drizin I
Gregg RJ
Scanio MJ
Shi L
Gross MF
Atkinson RN
Thomas JB
Johnson MS
Carroll WA
Marron BE
Chapman ML
Liu D
Krambis MJ
Shieh CC
Zhang X
Hernandez G
Gauvin DM
Mikusa JP
Zhu CZ
Joshi S
Honore P
Marsh KC
Roeloffs R
Werness S
Krafte DS
Jarvis MF
Faltynek CR
Kort ME
Source :
Bioorganic & medicinal chemistry [Bioorg Med Chem] 2008 Jun 15; Vol. 16 (12), pp. 6379-86. Date of Electronic Publication: 2008 May 06.
Publication Year :
2008

Abstract

The synthesis and pharmacological characterization of a novel furan-based class of voltage-gated sodium channel blockers is reported. Compounds were evaluated for their ability to block the tetrodotoxin-resistant sodium channel Na(v)1.8 (PN3) as well as the Na(v)1.2 and Na(v)1.5 subtypes. Benchmark compounds from this series possessed enhanced potency, oral bioavailability, and robust efficacy in a rodent model of neuropathic pain, together with improved CNS and cardiovascular safety profiles compared to the clinically used sodium channel blockers mexiletine and lamotrigine.

Details

Language :
English
ISSN :
1464-3391
Volume :
16
Issue :
12
Database :
MEDLINE
Journal :
Bioorganic & medicinal chemistry
Publication Type :
Academic Journal
Accession number :
18501613
Full Text :
https://doi.org/10.1016/j.bmc.2008.05.003